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Emerging natural and tailored perovskite-type mixed oxides-based catalysts for CO2 conversions

文献类型： 外文期刊

作者： Wu, Juan 1 ; Ye, Runping 2 ; Xu, Dong-Jie 3 ; Wan, Lingzhong 1 ; Reina, Tomas Ramirez 4 ; Sun, Hui 1 ; Ni, Ying 1 ; Zhou, Zhang-Feng 3 ; Deng, Xiaonan 1 ;

作者机构： 1.Anhui Acad Agr Sci, Inst Cotton, Hefei, Peoples R China

2.Nanchang Univ, Inst Appl Chem, Sch Chem & Chem Engn, Key Lab Jiangxi Prov Environm & Energy Catalysis, Nanchang, Peoples R China

3.Chinese Acad Sci, Fujian Inst Res Struct Matter, Key Lab Coal Ethylene Glycol & Its Related Technol, Fuzhou, Peoples R China

4.Univ Surrey, Dept Chem & Proc Engn, Guildford, England

5.Univ Seville CSIC, Mat Sci Inst, Dept Inorgan Chem, Seville, Spain

关键词： CO2 conversions; oxygen vacancies; dispersion of active metal; strong metal-support interactions; perovskite-type mixed oxide based catalysts

期刊名称：FRONTIERS IN CHEMISTRY （ 影响因子：5.545； 五年影响因子：5.869 ）

ISSN： 2296-2646

年卷期： 2022 年 10 卷

页码：

收录情况： SCI

摘要： The rapid economic and societal development have led to unprecedented energy demand and consumption resulting in the harmful emission of pollutants. Hence, the conversion of greenhouse gases into valuable chemicals and fuels has become an urgent challenge for the scientific community. In recent decades, perovskite-type mixed oxide-based catalysts have attracted significant attention as efficient CO2 conversion catalysts due to the characteristics of both reversible oxygen storage capacity and stable structure compared to traditional oxide-supported catalysts. In this review, we hand over a comprehensive overview of the research for CO2 conversion by these emerging perovskite-type mixed oxide-based catalysts. Three main CO2 conversions, namely reverse water gas shift reaction, CO2 methanation, and CO2 reforming of methane have been introduced over perovskite-type mixed oxide-based catalysts and their reaction mechanisms. Different approaches for promoting activity and resisting carbon deposition have also been discussed, involving increased oxygen vacancies, enhanced dispersion of active metal, and fine-tuning strong metal-support interactions. Finally, the current challenges are mooted, and we have proposed future research prospects in this field to inspire more sensational breakthroughs in the material and environment fields.

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